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Abstract The ~5 Myr PDS 70 is the only known system with protoplanets residing in the cavity of the circumstellar disk from which they formed, ideal for studying exoplanet formation and evolution within its natal environment. Here, we report the first spin constraint and C/O measurement of PDS 70b from Keck/KPIC high-resolution spectroscopy. We detected CO (3.8σ) and H₂O (3.5σ) molecules in the PDS 70b atmosphere via cross correlation, with a combined CO and H₂O template detection significance of 4.2σ. Our forward-model fits, using BT-Settl model grids, provide an upper limit for the spin rate of PDS 70b (<29 km s⁻¹). The atmospheric retrievals constrain the PDS 70b C/O ratio to ${0.28}_{-0.12}^{+0.20}$(<0.63 under 95% confidence level) and a metallicity [C/H] of ${-0.2}_{-0.5}^{+0.8}$dex, consistent with that of its host star. The following scenarios can explain our measured C/O of PDS 70b in contrast with that of the gas-rich outer disk (for which C/O ≳ 1). First, the bulk composition of PDS 70b might be dominated by dust+ice aggregates rather than disk gas. Another possible explanation is that the disk became carbon enrichedafterPDS 70b was formed, as predicted in models of disk chemical evolution and as observed in both very low-mass stars and older disk systems with JWST/MIRI. Because PDS 70b continues to accrete and its chemical evolution is not yet complete, more sophisticated modeling of the planet and the disk, and higher-quality observations of PDS 70b (and possibly PDS 70c), are necessary to validate these scenarios. 

Abstract We present the projected rotational velocity and molecular abundances for HD 33632 Ab obtained via Keck Planet Imager and Characterizer (KPIC) high-resolution spectroscopy. HD 33632 Ab is a nearby benchmark brown dwarf companion at a separation of ∼20 au that straddles the L–T transition. Using a forward-modeling framework with on-axis host star spectra, which provides self-consistent substellar atmospheric and retrieval models for HD 33632 Ab, we derive a projected rotational velocity of 53 ± 3 km s⁻¹and carbon monoxide and water mass fractions of logCO = −2.3 ± 0.3 and logH₂O = −2.7 ± 0.2, respectively. The inferred carbon-to-oxygen ratio (C/O = 0.58 ± 0.14), molecular abundances, and metallicity ([C/H] = 0.0 ± 0.2 dex) of HD 33632 Ab are consistent with its host star. Although detectable methane opacities are expected in L–T transition objects, we did not recover methane in our KPIC spectra, partly due to the highvsiniand to disequilibrium chemistry at the pressures to which we are sensitive. We parameterize the spin as the ratio of rotation to the breakup velocity, and compare HD 33632 Ab to a compilation of >200 very low-mass objects (M≲ 0.1M_⊙) that have spin measurements in the literature. There appears to be no clear trend for the isolated low-mass field objects versus mass, but a tentative trend is identified for low-mass companions and directly imaged exoplanets, similar to previous findings. A larger sample of close-in gas giant exoplanets and brown dwarfs will critically examine our understanding of their formation and evolution through rotation and chemical abundance measurements.